Search results for "Aerosol composition"
showing 5 items of 5 documents
A study on the sensitivities of simulated aerosol optical properties to composition and size distribution using airborne measurements
2014
We present a flexible framework to calculate the optical properties of atmospheric aerosols at a given relative humidity based on their composition and size distribution. The similarity of this framework to climate model parameterisations allows rapid and extensive sensitivity tests of the impact of uncertainties in data or of new measurements on climate relevant aerosol properties. The data collected by the FAAM BAe-146 aircraft during the EUCAARI-LONGREX and VOCALS-REx campaigns have been used in a closure study to analyse the agreement between calculated and measured aerosol optical properties for two very different aerosol types. The agreement achieved for the EUCAARI-LONGREX flights is…
Aircraft-based observation of meteoric material in lower-stratospheric aerosol particles between 15 and 68° N
2021
We analyse aerosol particle composition measurements from five research missions between 2014 and 2018 to assess the meridional extent of particles containing meteoric material in the upper troposphere and lower stratosphere (UTLS). Measurements from the Jungfraujoch mountaintop site and a low-altitude aircraft mission show that meteoric material is also present within middle- and lower-tropospheric aerosol but within only a very small proportion of particles. For both the UTLS campaigns and the lower- and mid-troposphere observations, the measurements were conducted with single-particle laser ablation mass spectrometers with bipolar-ion detection, which enabled us to measure the chemical c…
A numerical model of the cloud-topped planetary boundary-layer: influence of the physico-chemical properties of aerosol particles on the effective ra…
2000
The present investigation deals with the impact of different aeorosol types on the value of the effective radius of stratiform clouds. In several numerical sensitivity studies with the microphysical stratus model MISTRA, the aerosol composition was linearly changed from pure maritime to pure rural aerosol particles. Numerical results show that in environments with pure maritime aerosols, the effective radius is usually much larger than in continental regions. Values of the effective radius are also time-dependent with minima and maxima during day and night, respectively. In precipitating clouds, the effective radius might achieve values larger than 30 μm. In continental regions, the effecti…
Reactive species formed upon interaction of water with fine particulate matter from remote forest and polluted urban air
2020
Interaction of water with fine particulate matter leads to the formation of reactive species (RS) that may influence the aging, properties, and health effects of atmospheric aerosols. In this study, we explore the RS yields of fine PM from remote forest (Hyytiälä, Finland) and polluted urban air (Mainz, Germany and Beijing, China) and relate these yields to different chemical constituents and reaction mechanisms. Ultrahigh-resolution mass spectrometry was used to characterize organic aerosol composition, electron paramagnetic resonance (EPR) spectroscopy with a spin-trapping technique was used to determine the concentrations •OH, O2•−, and carbon- or oxygen-centered organic radicals, …
Particle chemical properties in the vertical column based on aircraft observations in the vicinity of Cape Verde Islands
2011
During the second Saharan Mineral Dust Experiment (SAMUM-2) field campaign, particles with geometric diameters (d) between ∼0.1 and 25 μm were collected on board of the Deutsches Zentrum für Luft- und Raumfahrt (German Aerospace Center, DLR) Falcon aircraft. Size, chemical composition and mixing state of aerosols sampled (spatially and vertically resolved) along the West African coastline and in the Cape Verde Islands region were determined by electron microscopy. A pronounced layer structure of biomass-burning aerosol and desert dust was present for all days during the sampling period from 23 January to 6 February. The aerosol composition of the small particles (d < 0.5 μm) was highly v…